IndiumV3, Main, Repository, bibRecord, 000068

Novel 9,9'-(1,3-Phenylene)bis-9H-carbazole-Containing Copolymers as Hole-Transporting and Host Materials for Blue Phosphorescent Polymer Light-Emitting Diodes

Identifieur interne : 000068 ( Main/Repository ); précédent : 000067; suivant : 000069

Novel 9,9'-(1,3-Phenylene)bis-9H-carbazole-Containing Copolymers as Hole-Transporting and Host Materials for Blue Phosphorescent Polymer Light-Emitting Diodes

Auteurs : RBID : Pascal:14-0101146

Descripteurs français

Pascal (Inist)
- Styrène copolymère, Styrène dérivé copolymère, Carbazole dérivé copolymère, Ether cyclique copolymère, Polymère redox, Préparation, Copolymérisation radicalaire, Propriété électrochimique, Stabilité thermique, Solution organique, Absorption optique, Photoluminescence, Réticulation photochimique, Copolymère réticulé, Résistance solvant, Polymère dopé, Iridium III Complexe, Matériau luminescent, Diode électroluminescente organique, Electroluminescence, Caractéristique courant tension, Lumière bleue, Rendement quantique, Etude expérimentale, Oxétane dérivé copolymère, Matériau transport trous.

English descriptors

KwdEn :
- Blue light, Carbazole derivative copolymer, Crosslinked copolymer, Cyclic ether copolymer, Doped polymer, Electrochemical properties, Electroluminescence, Experimental study, Iridium III Complexes, Luminescent material, Optical absorption, Organic light emitting diodes, Organic solution, Photochemical crosslinking, Photoluminescence, Preparation, Quantum yield, Radical copolymerization, Redox polymer, Solvent resistance, Styrene copolymer, Styrene derivative copolymer, Thermal stability, Voltage current curve.

Abstract

Novel photo-crosslinkable hole-transport and host materials incorporated into multilayer blue phosphorescent polymer light-emitting diodes (Ph-PLEDs) were demonstrated in this study. The oxetane-containing copolymers, which function as hole-transport layers (HTL), could be cured by UV irradiation in the presence of a cationic photoinitiator. The composition of the two monomers was varied to yield three different hole-transporting copolymers, [Poly(9,9'-(5-(((4-(7-(4-(((3-methyloxetan-3-yl)methoxy)methyl)phenyl)octan-3-yl)benz yl)oxy)methyl)-1,3-phenylene)bis(9H-carbazole)) (P(mCP-Ox)-I, -II, and -III)]. In addition, monomer 1 was copolymerized with styrene to produce copolymer P(mCP-Ph) as a host material for bis[2-(4,6-difluorophenyl)pyridinato-C²,N](picolinato)iridium(III) (Flrpic), a blue-emitting dopant. All mCP-based copolymers displayed high glass transition temperatures (T_g) of up to 130-140 °C and triplet energies of up to 3.00 eV. The blue Ph-PLEDs exhibited a maximum external quantum efficiency of 2.55%, in addition to a luminous efficiency of 8.75 cd A^-1 when using the device configuration of indium tin oxide/p-oly(3,4-ethylenedioxythiophene):poly(styrene sulfonate)/P(mCP-OX)-III/P(mCP-Ph):Flrpic(15wt%)/3,3?-[5?-[3-(3-pyridinyl)phenyl] [1,1?:3?,1?-terphenyl]-3,3?-diyl]bispyridine/LiF/Al. The device bearing P(mCP-Ox)-III HTL, containing the highest composition of mCP unit, exhibited better performance than the other devices, which is attributed to induction of more balanced charge carriers and carrier recombination in the emissive layer.

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Pascal:14-0101146

Le document en format XML

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<author><name>HYUN AH UM</name>
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<author><name>YONG JAE KIM</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Department of Information Display, Kyung Hee University, 26 Kyungheedae-ro</s1>
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<author><name>YOUNG HOON SON</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Department of Information Display, Kyung Hee University, 26 Kyungheedae-ro</s1>
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<country>Corée du Sud</country>
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<author><name>JOONG HWAN YANG</name>
<affiliation wicri:level="1"><inist:fA14 i1="03"><s1>LG Display, Co., LTD. 1007 Deogeon-ri, Wollong-myeon</s1>
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<author><name>GEESUNG CHAE</name>
<affiliation wicri:level="1"><inist:fA14 i1="03"><s1>LG Display, Co., LTD. 1007 Deogeon-ri, Wollong-myeon</s1>
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<author><name>JANG HYUK KWON</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Department of Information Display, Kyung Hee University, 26 Kyungheedae-ro</s1>
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<author><name>DONG HOON CHOI</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Chemistry, Research Institute for Natural Sciences, Korea University, 5 Anam-dong</s1>
<s2>Sungbuk-gu, Seoul 136-701</s2>
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<title level="j" type="abbreviated">J. polym. sci., Part A, Polym. chem.</title>
<title level="j" type="main">Journal of polymer science. Part A. Polymer chemistry</title>
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<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Blue light</term>
<term>Carbazole derivative copolymer</term>
<term>Crosslinked copolymer</term>
<term>Cyclic ether copolymer</term>
<term>Doped polymer</term>
<term>Electrochemical properties</term>
<term>Electroluminescence</term>
<term>Experimental study</term>
<term>Iridium III Complexes</term>
<term>Luminescent material</term>
<term>Optical absorption</term>
<term>Organic light emitting diodes</term>
<term>Organic solution</term>
<term>Photochemical crosslinking</term>
<term>Photoluminescence</term>
<term>Preparation</term>
<term>Quantum yield</term>
<term>Radical copolymerization</term>
<term>Redox polymer</term>
<term>Solvent resistance</term>
<term>Styrene copolymer</term>
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<keywords scheme="Pascal" xml:lang="fr"><term>Styrène copolymère</term>
<term>Styrène dérivé copolymère</term>
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<term>Ether cyclique copolymère</term>
<term>Polymère redox</term>
<term>Préparation</term>
<term>Copolymérisation radicalaire</term>
<term>Propriété électrochimique</term>
<term>Stabilité thermique</term>
<term>Solution organique</term>
<term>Absorption optique</term>
<term>Photoluminescence</term>
<term>Réticulation photochimique</term>
<term>Copolymère réticulé</term>
<term>Résistance solvant</term>
<term>Polymère dopé</term>
<term>Iridium III Complexe</term>
<term>Matériau luminescent</term>
<term>Diode électroluminescente organique</term>
<term>Electroluminescence</term>
<term>Caractéristique courant tension</term>
<term>Lumière bleue</term>
<term>Rendement quantique</term>
<term>Etude expérimentale</term>
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<front><div type="abstract" xml:lang="en">Novel photo-crosslinkable hole-transport and host materials incorporated into multilayer blue phosphorescent polymer light-emitting diodes (Ph-PLEDs) were demonstrated in this study. The oxetane-containing copolymers, which function as hole-transport layers (HTL), could be cured by UV irradiation in the presence of a cationic photoinitiator. The composition of the two monomers was varied to yield three different hole-transporting copolymers, [Poly(9,9'-(5-(((4-(7-(4-(((3-methyloxetan-3-yl)methoxy)methyl)phenyl)octan-3-yl)benz yl)oxy)methyl)-1,3-phenylene)bis(9H-carbazole)) (P(mCP-Ox)-I, -II, and -III)]. In addition, monomer 1 was copolymerized with styrene to produce copolymer P(mCP-Ph) as a host material for bis[2-(4,6-difluorophenyl)pyridinato-C<sup>2</sup>
,N](picolinato)iridium(III) (Flrpic), a blue-emitting dopant. All mCP-based copolymers displayed high glass transition temperatures (T<sub>g</sub>
) of up to 130-140 °C and triplet energies of up to 3.00 eV. The blue Ph-PLEDs exhibited a maximum external quantum efficiency of 2.55%, in addition to a luminous efficiency of 8.75 cd A<sup>-1</sup>
 when using the device configuration of indium tin oxide/p-oly(3,4-ethylenedioxythiophene):poly(styrene sulfonate)/P(mCP-OX)-III/P(mCP-Ph):Flrpic(15wt%)/3,3?-[5?-[3-(3-pyridinyl)phenyl] [1,1?:3?,1?-terphenyl]-3,3?-diyl]bispyridine/LiF/Al. The device bearing P(mCP-Ox)-III HTL, containing the highest composition of mCP unit, exhibited better performance than the other devices, which is attributed to induction of more balanced charge carriers and carrier recombination in the emissive layer.</div>
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<fC01 i1="01" l="ENG"><s0>Novel photo-crosslinkable hole-transport and host materials incorporated into multilayer blue phosphorescent polymer light-emitting diodes (Ph-PLEDs) were demonstrated in this study. The oxetane-containing copolymers, which function as hole-transport layers (HTL), could be cured by UV irradiation in the presence of a cationic photoinitiator. The composition of the two monomers was varied to yield three different hole-transporting copolymers, [Poly(9,9'-(5-(((4-(7-(4-(((3-methyloxetan-3-yl)methoxy)methyl)phenyl)octan-3-yl)benz yl)oxy)methyl)-1,3-phenylene)bis(9H-carbazole)) (P(mCP-Ox)-I, -II, and -III)]. In addition, monomer 1 was copolymerized with styrene to produce copolymer P(mCP-Ph) as a host material for bis[2-(4,6-difluorophenyl)pyridinato-C<sup>2</sup>
,N](picolinato)iridium(III) (Flrpic), a blue-emitting dopant. All mCP-based copolymers displayed high glass transition temperatures (T<sub>g</sub>
) of up to 130-140 °C and triplet energies of up to 3.00 eV. The blue Ph-PLEDs exhibited a maximum external quantum efficiency of 2.55%, in addition to a luminous efficiency of 8.75 cd A<sup>-1</sup>
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</fC03>
<fC03 i1="08" i2="X" l="SPA"><s0>Propiedad electroquímica</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>Stabilité thermique</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Thermal stability</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA"><s0>Estabilidad térmica</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="X" l="FRE"><s0>Solution organique</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="ENG"><s0>Organic solution</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="SPA"><s0>Solución orgánica</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE"><s0>Absorption optique</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG"><s0>Optical absorption</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA"><s0>Absorción óptica</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE"><s0>Photoluminescence</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG"><s0>Photoluminescence</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA"><s0>Fotoluminiscencia</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE"><s0>Réticulation photochimique</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="ENG"><s0>Photochemical crosslinking</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="SPA"><s0>Fotorreticulación</s0>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="X" l="FRE"><s0>Copolymère réticulé</s0>
<s2>NK</s2>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="ENG"><s0>Crosslinked copolymer</s0>
<s2>NK</s2>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="SPA"><s0>Copolímero reticulado</s0>
<s2>NK</s2>
<s5>14</s5>
</fC03>
<fC03 i1="15" i2="X" l="FRE"><s0>Résistance solvant</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="X" l="ENG"><s0>Solvent resistance</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="X" l="SPA"><s0>Resistencia a los disolventes</s0>
<s5>15</s5>
</fC03>
<fC03 i1="16" i2="X" l="FRE"><s0>Polymère dopé</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="ENG"><s0>Doped polymer</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="SPA"><s0>Polímero dopado</s0>
<s5>16</s5>
</fC03>
<fC03 i1="17" i2="X" l="FRE"><s0>Iridium III Complexe</s0>
<s1>SEC</s1>
<s2>NC</s2>
<s2>NA</s2>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="ENG"><s0>Iridium III Complexes</s0>
<s1>SEC</s1>
<s2>NC</s2>
<s2>NA</s2>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="SPA"><s0>Iridio III Complejo</s0>
<s1>SEC</s1>
<s2>NC</s2>
<s2>NA</s2>
<s5>17</s5>
</fC03>
<fC03 i1="18" i2="X" l="FRE"><s0>Matériau luminescent</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="ENG"><s0>Luminescent material</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="SPA"><s0>Material luminescente</s0>
<s5>18</s5>
</fC03>
<fC03 i1="19" i2="3" l="FRE"><s0>Diode électroluminescente organique</s0>
<s5>19</s5>
</fC03>
<fC03 i1="19" i2="3" l="ENG"><s0>Organic light emitting diodes</s0>
<s5>19</s5>
</fC03>
<fC03 i1="20" i2="X" l="FRE"><s0>Electroluminescence</s0>
<s5>20</s5>
</fC03>
<fC03 i1="20" i2="X" l="ENG"><s0>Electroluminescence</s0>
<s5>20</s5>
</fC03>
<fC03 i1="20" i2="X" l="SPA"><s0>Electroluminiscencia</s0>
<s5>20</s5>
</fC03>
<fC03 i1="21" i2="X" l="FRE"><s0>Caractéristique courant tension</s0>
<s5>21</s5>
</fC03>
<fC03 i1="21" i2="X" l="ENG"><s0>Voltage current curve</s0>
<s5>21</s5>
</fC03>
<fC03 i1="21" i2="X" l="SPA"><s0>Característica corriente tensión</s0>
<s5>21</s5>
</fC03>
<fC03 i1="22" i2="X" l="FRE"><s0>Lumière bleue</s0>
<s5>22</s5>
</fC03>
<fC03 i1="22" i2="X" l="ENG"><s0>Blue light</s0>
<s5>22</s5>
</fC03>
<fC03 i1="22" i2="X" l="SPA"><s0>Luz azul</s0>
<s5>22</s5>
</fC03>
<fC03 i1="23" i2="X" l="FRE"><s0>Rendement quantique</s0>
<s5>23</s5>
</fC03>
<fC03 i1="23" i2="X" l="ENG"><s0>Quantum yield</s0>
<s5>23</s5>
</fC03>
<fC03 i1="23" i2="X" l="SPA"><s0>Rendimiento quántico</s0>
<s5>23</s5>
</fC03>
<fC03 i1="24" i2="X" l="FRE"><s0>Etude expérimentale</s0>
<s5>24</s5>
</fC03>
<fC03 i1="24" i2="X" l="ENG"><s0>Experimental study</s0>
<s5>24</s5>
</fC03>
<fC03 i1="24" i2="X" l="SPA"><s0>Estudio experimental</s0>
<s5>24</s5>
</fC03>
<fC03 i1="25" i2="X" l="FRE"><s0>Oxétane dérivé copolymère</s0>
<s2>NK</s2>
<s4>INC</s4>
<s5>41</s5>
</fC03>
<fC03 i1="26" i2="X" l="FRE"><s0>Matériau transport trous</s0>
<s4>INC</s4>
<s5>42</s5>
</fC03>
<fC07 i1="01" i2="X" l="FRE"><s0>Propriété optique</s0>
<s5>31</s5>
</fC07>
<fC07 i1="01" i2="X" l="ENG"><s0>Optical properties</s0>
<s5>31</s5>
</fC07>
<fC07 i1="01" i2="X" l="SPA"><s0>Propiedad óptica</s0>
<s5>31</s5>
</fC07>
<fC07 i1="02" i2="X" l="FRE"><s0>Propriété chimique</s0>
<s5>32</s5>
</fC07>
<fC07 i1="02" i2="X" l="ENG"><s0>Chemical properties</s0>
<s5>32</s5>
</fC07>
<fC07 i1="02" i2="X" l="SPA"><s0>Propiedad química</s0>
<s5>32</s5>
</fC07>
<fN21><s1>139</s1>
</fN21>
</pA>
</standard>
</inist>
</record>

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   |wiki=   *** parameter Area/wikiCode missing *** 
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   |texte=   Novel 9,9'-(1,3-Phenylene)bis-9H-carbazole-Containing Copolymers as Hole-Transporting and Host Materials for Blue Phosphorescent Polymer Light-Emitting Diodes
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Novel 9,9'-(1,3-Phenylene)bis-9H-carbazole-Containing Copolymers as Hole-Transporting and Host Materials for Blue Phosphorescent Polymer Light-Emitting Diodes

Novel 9,9'-(1,3-Phenylene)bis-9H-carbazole-Containing Copolymers as Hole-Transporting and Host Materials for Blue Phosphorescent Polymer Light-Emitting Diodes

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